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] |
excitonic
photoluminescence
and
band-gap
engineering
of
wide-gap
p-type
oxychalcogenide epitaxial films of LnCuOCh (Ln = La, Pr, and Nd; Ch = S or Se)
semiconductor alloys, J. Appl. Phys. 94 (2003) 5805–5808.
https://doi.org/10.1063/1.1618932.
[149] B. Medasani, M.L. Sushko, K.M. Rosso, D.K. Schreiber, S.M. Bruemmer, Temperature
Dependence of Self-diffusion in Cr2O3 from First Principles, The Journal of Physical | [
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https://doi.org/10.1063/1.1584074. | [
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] |
https://doi.org/10.1063/1.1584074.
[179] A.N. Banerjee, C.K. Ghosh, K.K. Chattopadhyay, Effect of excess oxygen on the
electrical properties of transparent p-type conducting CuAlO2+x thin films, Sol. Energy
Mater. Sol. Cells 89 (2005) 75–83. https://doi.org/10.1016/j.solmat.2005.01.003.
Figure 1. Band gap engineering of TCO material. Visible photons don't have enough energy to
excite electrons directly from the valence band to conduction band. Still, they have sufficient | [
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] |
excite electrons directly from the valence band to conduction band. Still, they have sufficient
energy to excite electrons from donor level to conduction band (in n-type TCO) or holes from the
acceptor level to valence band (in p-type TCO). The symbol (✓) and (×) represents the allowed
and forbidden transition.
Figure 2. Transmittance spectrum of TCO material.
Figure 3. Band structure overview of n-type and p-type material with degenerate doping, | [
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] |
Figure 3. Band structure overview of n-type and p-type material with degenerate doping,
illustrating the BM-shift, Fermi-level (EFL), vacuum level (EVL), fundamental band gap (Eg), and
secondary band gap (Esg). The dark blue shading portion represents the occupied energy states,
while empty one is unoccupied energy levels.
Figure 4. Schematic overview of CMVB technique [42]. Energy levels are not to scale.
Figure 5. Evolution of publications on p-type TCO materials. | [
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] |
Figure 5. Evolution of publications on p-type TCO materials.
Figure 6. Variation in electrical conductivity of Mg-doped CuScO2+y thin film as a function of
oxygen intercalation pressures [67].
Figure 7. Variation in electrical conductivity (σ), carrier concentration (n) and mobility (μ) of
ZnCo2O4 thin films as a function of oxygen partial pressure ratio [86].
Figure 8. Resistivity, mobility, and carrier concentration of NiO thin films with varying Cu-
content [98]. | [
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] |
content [98].
Figure 9. Changes in electrical resistivity, carrier type and carrier concentration of Ga-doped
SnO2 thin films [62].
Figure 10. Changes in resistivity (ρ), Hall mobility (μ), and carrier concentrations of Eu-doped
SnO2 thin films with varying Eu molar concentration [130].
(a) (b)
Figure 11. (a) Resistivity and hole density and (b) mobility of Cu2O thin films with LTB-Cu2O | [
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] |
Figure 11. (a) Resistivity and hole density and (b) mobility of Cu2O thin films with LTB-Cu2O
as a function of oxygen flow rates.
Figure 12. Optical transmission spectra of (a) Cr2O3, (b) Mg:Cr2O3, and (c) Mg,N:Cr2O3 thin
films deposited with precursor ratios of Cr:Mg 9:1 and Cr:N 1:4. The inset shows a cross-section
SEM image to measure film thickness [152].
Figure 13. The room temperature electrical conductivity of Cr2O3 thin films (deposited from | [
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] |
Figure 13. The room temperature electrical conductivity of Cr2O3 thin films (deposited from
various sources) measured at different post-annealing oxygen pressures [153].
Figure 14. Optical transmittance spectra of Al2O3 substrate and V2O3 thin films of varying
thicknesses. The inset illustrates the images of the Al2O3 substrate and V2O3 thin films with
different thicknesses [169].
Figure 15. ABO2 crystal lattice: (a) stoichiometric structure. (b & c) non-stoichiometric with | [
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] |
Figure 15. ABO2 crystal lattice: (a) stoichiometric structure. (b & c) non-stoichiometric with
excess oxygen: (b) occupying A and B cation sites (creates four holes, p-type), (c) occupying
interstitial sites (forms O2-, creates two holes, p-type).
Table 1: Cu-based materials as p-type TCO and their respective optoelectronic parameters.
Material
Deposition
technique
used
Thickness
(nm)
Substrate used
Average optical
Transmittance
(%)
Optical
band
gap
(eV)
Electrical
conductivity | [
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] |
Average optical
Transmittance
(%)
Optical
band
gap
(eV)
Electrical
conductivity
(S/cm)
Carrier
conc
(/cm3)
Hall
Mobility
(cm2/V-s)
Reference
CuAlO2
PLD
500
Sapphire
70
3.5
1
1.3 × 1017
10.4
[42]
CuGaO2
PLD
500
Sapphire
80
3.6
0.063
1.7 × 1018
0.23
[49]
Sn: CuInO2
PLD
280
Sapphire
< 50
3.9
3.8×10-3
-
-
[46]
Ca:
CuInO2
PLD
170
Sapphire
< 50
~3.9
2.83×10-3
-
-
[46]
CuScO2+x
Sputtering
110
Silica
40
3.3
15-30
-
-
[47]
CuY1-xCaxO2
Thermal co- | [
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] |
-
-
[46]
CuScO2+x
Sputtering
110
Silica
40
3.3
15-30
-
-
[47]
CuY1-xCaxO2
Thermal co-
evaporation
240
MgO
40-50
3.5
1
-
-
[48]
CuCr1-xMgxO2
RF-
sputtering
250
Quartz
30
3.1
220
-
-
[45]
Cu-deficient
CuCrO2
spray
pyrolysis
80
Glass
55
3
1-12
-
0.006
[70]
Mg, N:
CuCrO2
RF-
sputtering
150
Quartz
69.1
3.52
277.7
1.18×1021
0.006
[71]
Sn:CuNi1-
xSbxO2
RF-
sputtering
150-200
Fused silica
60
3.4
0.05
-
-
[72]
K-doped
SrCu2O2
PLD
200 | [
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] |
RF-
sputtering
150-200
Fused silica
60
3.4
0.05
-
-
[72]
K-doped
SrCu2O2
PLD
200
SiO2 glass
⁓ 70
3.3
4.8×10-2
6.13×1017
0.46
[50]
CuCrO2+x
Combustion
75
ITO
80-90
3.0
0.14
3.8 × 1018
0.23
[73]
CuCrO2
CVD
75-85
Boro
aluminosilicate
glass
60-65
3.2
50
9.3 × 1018
-1.5 × 1016
0.65-5
[74]
CuGaO2
RF-
sputtering
200
Fused quartz
60-70
3.47
0.0167
-
-
[75]
CuAlO2
Magnetron
Sputtering
400
Sapphire
75
3.85
1.05
2.5 × 1019
0.254
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] |
Magnetron
Sputtering
400
Sapphire
75
3.85
1.05
2.5 × 1019
0.254
[76]
Table 2: Ag-based materials as p-type TCO and their respective optoelectronic parameters.
Material
Deposition
technique
used
Thickness
(nm)
Substrate
used
Average optical
Transmittance
(%)
Optical
band gap
(eV)
Electrical
conductivity
(S/cm)
Carrier
conc
(/cm3)
Hall
Mobility
Reference
AgGaO2
PLD
200
Sapphire
50
4.12
3.2×10-4
-
-
[77]
AgCr1-xMgxO2 Spin Coating | [
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-0.17775003612041473,
0.07304675132036209,
-0.1663682460784912,
0.09368746727705002,
0.568466305732727,
-0.6732823252677917,
0.202867329120636,
-0.4731808006763458,
0.17469915747642517,
-0.21990782022476196,
-0.5340023636817932,
-1.0770246982574463,
0.5824359059333801,
-0.712958037853241,
-0.46997830271720886,
0.5341156125068665,
-0.3583349883556366,
-0.6641467809677124,
0.29794245958328247,
0.10946625471115112,
-0.22402937710285187,
0.6124260425567627,
0.0860736146569252,
0.4777602553367615,
0.10081855207681656,
-0.6221247315406799,
0.24964168667793274,
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0.1456703543663025,
0.5903619527816772,
-0.16859370470046997,
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0.04451549053192139,
-0.279323011636734,
-0.057499345391988754,
0.10337644815444946,
0.6707679629325867,
-0.4161991775035858,
0.12763695418834686,
0.1856420934200287,
0.3228518068790436,
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0.499172568321228,
-0.11424122750759125,
0.39252156019210815,
0.19040802121162415,
0.4291048049926758,
0.21277090907096863,
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-1.1960480213165283,
-0.20459917187690735,
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-0.16985556483268738,
-0.11671483516693115,
0.6267156600952148,
-0.38414129614830017,
0.5466119050979614,
0.22522130608558655,
-0.5498065948486328,
0.36163604259490967,
0.8374569416046143,
-0.559358537197113,
-0.06343643367290497,
0.19963155686855316,
0.2960212230682373,
-0.42122015357017517,
-0.19458052515983582,
-0.0923861637711525,
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-0.02503775805234909,
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0.14031274616718292,
0.4964376389980316,
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0.12834611535072327,
0.10378922522068024,
0.2656712830066681,
-0.43211182951927185,
-0.35502883791923523,
0.09000981599092484,
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0.07968872785568237,
0.12463240325450897,
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0.640052318572998,
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0.1911502480506897,
0.29449599981307983,
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-0.0027686655521392822,
0.38493412733078003,
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0.0035492770839482546,
0.09409730136394501,
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0.3552934229373932,
0.02521599270403385,
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0.5827075242996216,
0.5887463688850403,
0.24434514343738556,
0.04413989931344986,
-0.6199259161949158,
0.28018882870674133,
0.593619167804718,
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0.32853826880455017,
0.15088343620300293,
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0.17669591307640076,
0.1795082986354828,
0.40943264961242676,
0.10140956938266754,
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-0.07261524349451065,
-0.4025174081325531,
0.07530675828456879,
0.3123141825199127,
-0.020103927701711655,
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-0.3689703047275543,
0.21086403727531433,
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0.5824245810508728,
0.6973658800125122,
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-0.3301045298576355,
-0.03526933863759041,
-0.3575633764266968,
-0.5499283075332642,
0.36884117126464844,
-0.41554179787635803,
0.5318989753723145,
-0.027363702654838562,
0.19960705935955048,
-0.5379682183265686,
0.5059550404548645,
0.9806085824966431,
-0.4144050180912018,
-0.6260453462600708,
-0.16721409559249878,
0.44528138637542725,
-0.6073346138000488,
0.19821502268314362,
0.15835875272750854,
0.14236006140708923,
0.14512452483177185,
0.13727955520153046,
0.15562231838703156,
-0.30238431692123413,
0.06151536479592323,
-0.5148630738258362,
0.2596088647842407,
0.1584949791431427,
-0.2863481640815735,
0.40857747197151184,
-0.0613311342895031,
0.1577366292476654,
-0.3439069390296936,
-0.041259296238422394,
-0.10372762382030487,
-0.3248864710330963,
-0.04702690988779068,
-0.0506756491959095,
-0.17486579716205597,
0.2567715346813202,
0.40962594747543335,
-0.4365800619125366,
-0.05096052959561348,
-0.03996929153800011,
-0.0737343281507492,
-0.3363622725009918,
-0.00010668910545064136,
0.036622900515794754,
-0.20163457095623016,
0.32106658816337585,
-1.383344292640686,
0.055529072880744934,
0.03661452606320381,
0.28749173879623413,
0.03633861243724823,
-0.05792704597115517,
-0.08205308020114899,
-0.046514708548784256,
-0.5178208351135254,
0.2254473865032196,
0.5864389538764954,
-0.49824753403663635,
-0.6149908900260925,
-0.21721656620502472,
0.3540268838405609,
-0.15908482670783997,
-0.3992233872413635,
-0.2780262231826782,
0.7388587594032288,
0.30915260314941406,
0.008164240047335625,
-0.35961511731147766,
-0.2032860666513443,
0.6796053647994995,
-0.5349053144454956,
0.4632401466369629,
-0.7809209227561951,
-0.38330748677253723,
-0.298811137676239,
0.5423002243041992,
0.10055626183748245,
-1.0685731172561646,
0.11147910356521606,
-0.05890423059463501,
-0.4540436565876007,
0.7127768397331238,
0.7393165230751038,
0.7950912117958069,
-0.5021239519119263,
0.15357078611850739,
-0.43676239252090454,
0.2853963375091553,
-0.24318641424179077,
0.34444910287857056,
-0.5589195489883423,
-0.6149976849555969,
0.6722167134284973,
0.04276113212108612,
0.22094468772411346,
0.14824019372463226,
0.02164648100733757,
0.17672251164913177,
-0.5355127453804016,
0.14232498407363892,
0.270073264837265,
0.3389861285686493,
-1.0123927593231201,
-0.6609715223312378,
-0.3005119562149048,
0.14121021330356598,
0.17167718708515167,
-0.00780797703191638,
-0.04111335054039955,
0.00860107596963644,
-0.6097029447555542,
0.7141180634498596,
0.6103902459144592,
-0.9244935512542725,
0.3981618881225586,
-0.2154504507780075,
0.2758919894695282,
-0.14989878237247467,
0.23325243592262268,
-0.40886521339416504,
-0.04690477252006531,
-0.15386082231998444,
-0.1559450328350067,
0.4086501896381378,
-0.4688108265399933,
-0.29341837763786316,
0.17688676714897156,
0.04784727096557617,
0.3681999742984772,
0.23935437202453613,
-0.014931854791939259,
0.49263766407966614,
0.6449189782142639,
-0.012254157103598118,
-0.7162030935287476,
0.39032143354415894,
-0.37251773476600647,
0.17507071793079376,
-0.07307738065719604,
-0.263629674911499,
0.4193492829799652,
-0.34103137254714966,
-0.22214950621128082,
0.5327053666114807,
0.2859886884689331,
0.524859607219696,
-0.2115500122308731,
-0.04969364032149315,
-0.2525211572647095,
0.8614948987960815,
-0.05503523349761963,
0.7921324968338013,
-0.34107324481010437,
-0.14290226995944977,
-0.44490301609039307,
0.3876767158508301,
0.24070070683956146,
-0.13075824081897736,
-0.2566099166870117,
0.2627636790275574,
-0.26223114132881165,
-0.04467278718948364,
-0.6476718187332153,
-0.48175376653671265,
-0.7730597257614136,
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0.20889760553836823,
-0.2981216013431549,
-0.1099739745259285,
0.16821318864822388,
0.16978904604911804,
0.7826240658760071,
-0.03486856818199158,
0.20602218806743622,
-0.8931190967559814,
-0.19892334938049316,
0.12649574875831604,
0.02999831736087799,
-0.18909648060798645,
-0.3291403353214264,
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-0.2750520706176758,
-0.12005728483200073,
0.730186939239502,
-0.38057741522789,
-0.48875510692596436,
0.20321476459503174,
0.1939401477575302,
-0.06802168488502502,
0.26651057600975037,
-0.5659340023994446,
0.3337804079055786,
-0.2706587612628937,
-0.4009215831756592,
0.4658011496067047,
-0.4281976819038391,
0.2958666682243347,
0.1576322317123413,
-0.04424433037638664,
-0.07779508829116821,
0.5257987976074219,
-0.39536574482917786,
-0.0053450316190719604,
0.03806053474545479,
-0.19154098629951477,
-0.5400667786598206,
-0.11704262346029282,
0.35561373829841614,
0.444713830947876,
0.46101444959640503,
0.1455708146095276,
0.46336013078689575,
0.23180055618286133,
0.7888078093528748,
-0.686931848526001,
0.6800219416618347,
-0.3031374514102936,
0.7158717513084412,
-0.8165802359580994,
-0.17338572442531586,
0.5703751444816589,
0.10987183451652527,
-0.2759365141391754,
-0.3109062910079956,
0.38261163234710693,
-0.38395312428474426,
0.23251843452453613,
-0.3807693421840668,
-0.18240267038345337,
-0.1714634895324707,
-0.2711721360683441,
-0.9786543250083923,
0.4478992819786072,
0.3409414291381836,
0.04181043431162834,
-0.2108001857995987,
0.47189703583717346,
-0.20247825980186462,
0.0801304504275322,
0.13812074065208435,
0.07821270078420639,
-0.035742275416851044,
-0.09923845529556274,
0.521859884262085,
-0.28571924567222595,
0.18620099127292633,
-0.47147342562675476,
0.5881238579750061,
-0.422778844833374,
-0.28090572357177734,
-0.11305492371320724,
-0.38650280237197876,
-0.36793282628059387,
0.05374641343951225,
0.1090795174241066,
0.6340720653533936,
-0.048914022743701935,
-0.39037418365478516,
-0.8949914574623108,
0.19582627713680267,
0.05852457508444786,
-0.6925776600837708,
0.024135854095220566,
-0.11223386228084564,
-0.20390887558460236,
-0.5842247605323792,
-0.27023595571517944,
-0.15283484756946564,
0.17262965440750122,
0.23446966707706451
] |
Reference
AgGaO2
PLD
200
Sapphire
50
4.12
3.2×10-4
-
-
[77]
AgCr1-xMgxO2 Spin Coating
120
Sapphire
60
3.66
67.7×10-3
1.25×1017
50
[79]
Ag-deficient
AgInGaO2
Reactive
Evaporation
-
Glass
substrate
25
3.77
61
2.2×1018
0.017
[80]
Table 3: Spinel materials as p-type TCO and their respective optoelectronic parameters.
Material
Deposition
technique
used
Thickness
(nm)
Substrate
used
Average optical
Transmittance
(%)
Optical
band gap
(eV)
Electrical | [
0.0369311086833477,
0.3114086985588074,
0.6671746373176575,
0.11777326464653015,
-0.019020698964595795,
0.1307554543018341,
0.19272193312644958,
-0.3957831859588623,
0.05099079757928848,
-0.036476437002420425,
-0.006917736958712339,
0.596156895160675,
-0.21582284569740295,
0.3273037374019623,
0.25898444652557373,
1.0819233655929565,
0.49808380007743835,
0.41626882553100586,
0.13968341052532196,
-0.9610111117362976,
0.0006824788288213313,
-0.23188237845897675,
0.9448214173316956,
-0.41438207030296326,
0.1190449669957161,
0.33129218220710754,
0.324592262506485,
0.17050573229789734,
0.081047922372818,
0.1283928006887436,
-0.15217213332653046,
0.9119259715080261,
0.06296103447675705,
0.010750606656074524,
0.7443227767944336,
0.10632089525461197,
0.036385677754879,
0.10091497004032135,
-0.036844104528427124,
-0.4498843252658844,
-0.05609968677163124,
-0.24746090173721313,
0.009971557185053825,
0.7167692184448242,
-0.28583982586860657,
0.028837110847234726,
-1.1600362062454224,
0.18244816362857819,
-0.37606310844421387,
0.056511491537094116,
0.13988026976585388,
0.25260621309280396,
0.39912256598472595,
0.14287132024765015,
-0.02927514724433422,
0.23651552200317383,
-0.4600711762905121,
-0.36962175369262695,
0.21082229912281036,
-0.2767907381057739,
0.028322415426373482,
0.09498608857393265,
-0.2883032560348511,
0.4505448639392853,
-0.22827988862991333,
0.5480502843856812,
-0.10360575467348099,
-0.13680781424045563,
-0.1906963586807251,
0.11187859624624252,
0.5618899464607239,
0.23424196243286133,
-0.03991860896348953,
0.06360111385583878,
-0.09746559709310532,
0.14231091737747192,
-0.3618835508823395,
0.0019463341450318694,
0.2899535298347473,
0.10019026696681976,
0.3692830502986908,
-0.27348005771636963,
0.5994595289230347,
-0.0807945504784584,
0.16961459815502167,
0.4020213186740875,
-0.1196671798825264,
0.30833572149276733,
-0.3996412456035614,
0.8335237503051758,
-0.22822099924087524,
-0.07882917672395706,
0.4035460948944092,
0.9103800654411316,
-0.09775985032320023,
-0.2234850376844406,
-0.5076627731323242,
-0.241230770945549,
0.584300696849823,
0.20837539434432983,
-0.10620146989822388,
-0.12212073802947998,
-0.34271755814552307,
0.04463934525847435,
-0.35826343297958374,
-0.16805852949619293,
-0.8569225072860718,
-0.7099042534828186,
-0.38187259435653687,
0.2352728694677353,
-0.7334244251251221,
0.09411099553108215,
-0.40895935893058777,
-0.2081713080406189,
-0.1834416538476944,
0.01879633218050003,
-0.052728064358234406,
-0.11171219497919083,
0.4593679904937744,
0.6625317931175232,
0.28642791509628296,
0.8169399499893188,
-0.4242081344127655,
0.20918476581573486,
0.40196943283081055,
0.37200990319252014,
0.5925165414810181,
0.6956415176391602,
-0.2259557992219925,
0.6493331789970398,
0.06145196035504341,
0.7523745894432068,
-0.09610206633806229,
0.008149058558046818,
-0.2437705248594284,
-0.7450153827667236,
0.009412571787834167,
-0.18378369510173798,
0.174273282289505,
0.4219813346862793,
-0.17000408470630646,
-0.7314910292625427,
-0.48963481187820435,
-0.12414154410362244,
0.2109615057706833,
-0.3487507700920105,
0.17269267141819,
-0.018054088577628136,
-0.38021084666252136,
0.540472686290741,
-0.0036982677411288023,
-0.4826210141181946,
-0.4072815477848053,
0.23271356523036957,
-0.5754106640815735,
-0.10840867459774017,
-0.25846147537231445,
-0.019995063543319702,
-0.46571293473243713,
-0.09663853049278259,
0.3322308659553528,
0.19780558347702026,
-0.6637458205223083,
0.2943434417247772,
0.6502013802528381,
0.2679292559623718,
0.25117236375808716,
0.2200736105442047,
-0.13006407022476196,
0.11281958967447281,
0.1370478719472885,
-0.3810182511806488,
-0.4198305308818817,
-0.004439015407115221,
-0.5811867117881775,
0.296927809715271,
0.17057664692401886,
0.24017906188964844,
0.02996319904923439,
-0.01849200204014778,
-0.6871726512908936,
-0.3601173758506775,
0.07087778300046921,
0.02354508824646473,
0.3244103789329529,
0.39972206950187683,
0.8386900424957275,
0.06866537034511566,
0.32347825169563293,
0.10329880565404892,
-0.3168542981147766,
-0.06152941659092903,
0.8221940994262695,
-0.8011321425437927,
1.340131163597107,
-0.03870711848139763,
-0.41019031405448914,
0.4622938930988312,
-0.26257073879241943,
0.22368106245994568,
0.026054929941892624,
0.4893445372581482,
0.5333532094955444,
-0.5407243967056274,
-0.6595460176467896,
-0.12072562426328659,
0.11064180731773376,
0.05952613428235054,
0.07895771414041519,
-0.08214506506919861,
0.34813830256462097,
-0.3427796959877014,
-0.3697202503681183,
-0.4049178957939148,
0.35221293568611145,
-0.3169611990451813,
0.2965441942214966,
0.0421619676053524,
0.2828068733215332,
-0.30583828687667847,
0.7960325479507446,
-0.25075027346611023,
0.36160245537757874,
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] |
(nm)
Substrate
used
Average optical
Transmittance
(%)
Optical
band gap
(eV)
Electrical
conductivity
(S/cm)
Carrier
conc
(/cm3)
Hall
Mobility
(cm2/V-s)
Reference
NiCo2O4
Spin Casting
100
Sapphire
90
-
16.7
-
-
[81]
ZnRh2O4
RFMS
-
Silica glass
-
2.1
0.7
-
-
[82]
ZnCo2O4
RFMS
400
Silica glass
55
2.63
1.2
2.81×1020
0.2
[86]
ZnIr2O4
PLD
100-300
Quartz and
sapphire
60
2.97
2.09-3.39
-
-
[82]
ZnCo2O4
PLD
100-200
Sapphire
-
2.3
21.8
2.6×1016- | [
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0.03620559349656105,
0.9107130765914917,
0.1508307009935379,
0.4015338718891144,
0.18867872655391693,
0.26223933696746826,
-0.0008561246795579791,
-0.02797969989478588,
1.1398406028747559,
-0.42008867859840393,
0.12893933057785034,
-0.4941021800041199,
0.5764399766921997,
-0.489407479763031,
-0.09715660661458969,
-0.4468003809452057,
-0.3886672854423523,
-0.510953426361084,
0.24966971576213837,
0.07895342260599136,
0.12139527499675751,
-0.13090719282627106,
-1.050391674041748,
-1.1523222923278809,
0.06339161098003387,
0.07515943795442581,
-0.5514801144599915,
0.05702116712927818,
-0.11312565207481384,
-0.16626232862472534,
-0.20675724744796753,
0.06727250665426254,
-0.2244732528924942,
0.08819736540317535,
0.1451057493686676
] |
sapphire
60
2.97
2.09-3.39
-
-
[82]
ZnCo2O4
PLD
100-200
Sapphire
-
2.3
21.8
2.6×1016-
1.49×1020
0.12-0.6
[91]
ZnCo2O4
Spin coating
120
Glass
55
3.95-3.99
0.4×10-3-
0.6×10-2
5.57×1012-
4.29 ×1014
-
[89]
ZnGa2O4
MOCVD
100
Sapphire
80
5.1
7.6×10-4
1.6 ×1015
7-10
[90]
Table 4: Binary oxide materials as p-type TCO and their respective optoelectronic parameters.
Material
Deposition
technique
used
Thickness
(nm)
Substrate used
Average optical
Transmittance
(%) | [
0.5958392024040222,
0.12476726621389389,
0.17293132841587067,
0.24950817227363586,
-0.07622615993022919,
0.2251480519771576,
0.28032875061035156,
-0.4357975423336029,
0.06881317496299744,
0.12021548300981522,
-0.05939274653792381,
0.7584690451622009,
-0.006975424941629171,
0.30545517802238464,
0.13814884424209595,
0.9583547711372375,
0.8882015943527222,
0.3931805491447449,
0.11157584190368652,
-0.7892462015151978,
0.1939702033996582,
0.03931475430727005,
1.111911416053772,
-0.19398429989814758,
-0.19665494561195374,
0.14685341715812683,
0.23005631566047668,
-0.3176042437553406,
0.2923681139945984,
0.6207826733589172,
-0.09690627455711365,
0.9122048020362854,
0.020749079063534737,
-0.03773783519864082,
0.6892873644828796,
-0.15610326826572418,
-0.21694381535053253,
-0.13205116987228394,
-0.13005104660987854,
-0.4802570641040802,
0.2687933146953583,
-0.5073829889297485,
0.32145822048187256,
0.48090335726737976,
-0.1675778329372406,
0.12451618909835815,
-1.2071726322174072,
0.07981058210134506,
-0.1283075362443924,
-0.0501900352537632,
0.20576342940330505,
0.2129683643579483,
0.25370216369628906,
0.31210169196128845,
0.3058871328830719,
0.5631865859031677,
-1.006017804145813,
-0.14737819135189056,
0.23240838944911957,
0.3590543270111084,
0.35381603240966797,
0.15278860926628113,
-0.5151153206825256,
0.7179499864578247,
-0.054368674755096436,
0.5432243943214417,
0.1276213377714157,
-0.03509723022580147,
-0.4842429757118225,
0.026575816795229912,
0.6147652864456177,
-0.037493184208869934,
0.33260834217071533,
0.09627056866884232,
-0.4220763146877289,
0.45490285754203796,
-0.3503163158893585,
-0.11662973463535309,
0.28345516324043274,
-0.07398319989442825,
0.0741698294878006,
-0.03613070771098137,
0.8708381652832031,
0.39846983551979065,
0.12079782038927078,
-0.2352287918329239,
-0.1474917232990265,
0.27198129892349243,
-0.2012879103422165,
0.5333048105239868,
-0.46443694829940796,
-0.255769282579422,
0.4378088116645813,
0.8727961778640747,
-0.2823750674724579,
-0.4875270426273346,
-1.0060291290283203,
-0.20507702231407166,
0.5305174589157104,
0.026384597644209862,
-0.09221025556325912,
0.005825249012559652,
-0.20508772134780884,
0.13584832847118378,
-0.6736916899681091,
-0.336819052696228,
-0.7180457711219788,
-0.5851314067840576,
-0.3333730697631836,
0.2584315836429596,
-0.9524393677711487,
-0.13419906795024872,
-0.3069498538970947,
-0.14830054342746735,
-0.34791454672813416,
-0.035557717084884644,
0.04357152804732323,
-0.09642201662063599,
0.38609838485717773,
0.49188628792762756,
0.3256698548793793,
0.5273152589797974,
-0.16599901020526886,
0.43790772557258606,
0.3646993637084961,
0.46772411465644836,
0.783048152923584,
0.8323045969009399,
-0.25121060013771057,
0.20076334476470947,
0.03744330257177353,
1.0399000644683838,
-0.5308105945587158,
-0.060952410101890564,
-0.10983540862798691,
-1.0445866584777832,
0.32505831122398376,
-0.3894643485546112,
-0.1343679130077362,
0.5012074112892151,
-0.09288140386343002,
-0.20439155399799347,
-0.38431045413017273,
-0.2133471816778183,
-0.12121693044900894,
-0.05215811729431152,
0.3492693305015564,
0.31846296787261963,
-0.40533021092414856,
0.03794815018773079,
-0.05377116799354553,
-0.23880061507225037,
-0.31326788663864136,
-0.14972034096717834,
-0.48547831177711487,
-0.26065659523010254,
-0.06453416496515274,
0.190773144364357,
-0.20043335855007172,
0.04556669294834137,
-0.431534081697464,
0.09720151871442795,
-0.16289661824703217,
0.07863178104162216,
0.45118579268455505,
0.003924231510609388,
0.37690240144729614,
-0.02626178413629532,
-0.2684228718280792,
0.362020879983902,
0.0688747763633728,
0.14376559853553772,
-0.5202024579048157,
0.6312299370765686,
-0.7112365961074829,
-0.04586746543645859,
0.2011432945728302,
0.7797300219535828,
0.03059963509440422,
-0.24445024132728577,
-0.7692245244979858,
-0.3987879753112793,
-0.07484356313943863,
0.12083747237920761,
0.4745931327342987,
0.8838012218475342,
0.9682292938232422,
0.4623439311981201,
-0.17896898090839386,
0.04057643562555313,
-0.05323095992207527,
-0.06798555701971054,
0.3798462450504303,
-0.7373251914978027,
0.8067156672477722,
-0.04991568252444267,
-0.1411575824022293,
0.14652593433856964,
-0.383873850107193,
0.5177581310272217,
0.10516004264354706,
0.19287194311618805,
0.475708931684494,
-0.32984602451324463,
-0.7199698686599731,
-0.1510254144668579,
0.20643562078475952,
-0.17943209409713745,
-0.22105729579925537,
0.05924850329756737,
0.36557283997535706,
-0.34517091512680054,
-0.24729758501052856,
0.036213915795087814,
0.09633657336235046,
0.11014353483915329,
0.20930857956409454,
-0.07182510942220688,
0.24509820342063904,
-0.17602546513080597,
0.729040265083313,
-0.17433829605579376,
0.45489412546157837,
0.5225445628166199,
-0.4148922860622406,
0.9452540874481201,
0.5104841589927673,
-0.193388894200325,
-0.08363646268844604,
-0.17242436110973358,
-0.2595198452472687,
-0.3647290766239166,
0.4000531733036041,
0.11944559216499329,
0.720544695854187,
0.16762372851371765,
-0.1698608696460724,
0.14210596680641174,
0.8234435319900513,
-0.4151249825954437,
0.5639997720718384,
0.043788641691207886,
-0.47095391154289246,
0.3838709890842438,
0.44928789138793945,
-0.40844985842704773,
0.025366369634866714,
0.2524473965167999,
-0.16536085307598114,
-0.24364954233169556,
0.377613365650177,
-0.039414118975400925,
-0.11324219405651093,
-0.4377540647983551,
-0.5011880993843079,
-0.1151779517531395,
0.1173226535320282,
-0.4253743886947632,
-0.15842103958129883,
-0.1018386259675026,
-0.4363834261894226,
-0.2575168013572693,
0.2891858220100403,
-0.17747069895267487,
0.056167811155319214,
-0.3733085095882416,
-0.8501810431480408,
-0.12500590085983276,
0.6430197954177856,
0.030829744413495064,
-0.022634131833910942,
0.48100072145462036,
-0.649057149887085,
-0.0859144851565361,
-0.24007008969783783,
-0.511326014995575,
-0.4401519000530243,
0.4979928433895111,
-0.7184517979621887,
-0.377156525850296,
0.5038995146751404,
0.4873464107513428,
0.916100800037384,
-0.04705846309661865,
-1.0476222038269043,
-0.16407325863838196,
0.1096365824341774,
-0.6890836954116821,
-0.7141215205192566,
-1.1850873231887817,
-0.39754629135131836,
0.5365262031555176,
-0.35226914286613464,
-0.91371089220047,
0.18193094432353973,
0.2991185188293457,
-0.5777977705001831,
0.3679683804512024,
0.5144582390785217,
-0.27621492743492126,
0.13752709329128265,
0.21742883324623108,
-0.3242948055267334,
0.037417422980070114,
0.016479382291436195,
-0.9204720258712769,
-0.5113703012466431,
-0.26878413558006287,
-5.567597389221191,
0.35547634959220886,
-0.22876355051994324,
0.23812980949878693,
-0.2331559807062149,
-0.22719232738018036,
1.0019387006759644,
0.001794522744603455,
0.559334933757782,
-0.5661177039146423,
-0.2622827887535095,
0.3293335735797882,
-0.14794088900089264,
0.33084341883659363,
0.2271249145269394,
1.1025936603546143,
0.6432151198387146,
-0.5195925235748291,
0.5889621376991272,
0.05909573659300804,
0.6533387899398804,
-0.028004013001918793,
-0.2625442147254944,
0.22998683154582977,
0.36596402525901794,
-0.05208278074860573,
-0.4830981492996216,
0.2278539091348648,
-0.30636271834373474,
-0.14246857166290283,
-0.22585661709308624,
-0.07295346260070801,
-0.4578140377998352,
-0.06016071140766144,
0.36519360542297363,
0.06552590429782867,
0.7568381428718567,
-0.13535824418067932,
0.12119432538747787,
-0.4542888402938843,
0.6153822541236877,
0.5218691825866699,
0.12629002332687378,
0.06096109002828598,
0.5112438201904297,
0.3476925790309906,
-0.48099076747894287,
-0.12902209162712097,
0.04960542544722557,
0.5129076838493347,
-0.40779006481170654,
-0.6922464370727539,
0.2861153781414032,
-0.020436210557818413,
-0.11067570000886917,
0.343631386756897,
0.05931860953569412,
0.8536614179611206,
-0.5691276788711548,
0.19886183738708496,
-0.7122785449028015,
-0.035508062690496445,
0.1415843814611435,
-0.7786152362823486,
-0.3731015920639038,
0.10399419069290161,
-1.3235470056533813,
-0.24316725134849548,
0.4535771906375885,
-0.023988785222172737,
-0.48111599683761597,
0.2688923478126526,
-0.12763340771198273,
-0.48100709915161133,
0.5057307481765747,
-0.1626923531293869,
0.2039840817451477,
0.03995359316468239,
-0.5640071034431458,
0.3773134648799896,
0.027909623458981514,
-0.4163193106651306,
-0.08686669915914536,
0.3885703682899475,
0.14881184697151184,
-0.5454225540161133,
0.16950437426567078,
-0.29860520362854004,
-0.13652287423610687,
0.48184674978256226,
0.4856911301612854,
-0.27040690183639526,
-0.015177044086158276,
0.04326570779085159,
0.3095867931842804,
-0.42433053255081177,
0.6848623156547546,
-0.3504990041255951,
0.29085564613342285,
0.008532480336725712,
0.23253126442432404,
-0.3098047077655792,
-0.03351323679089546,
-1.1806352138519287,
-0.40890708565711975,
0.15634752810001373,
-0.2446565181016922,
0.01795242540538311,
0.3701620399951935,
-0.16507621109485626,
0.21630574762821198,
-0.24317236244678497,
-0.6276379227638245,
0.2213253676891327,
0.6918284296989441,
-0.6947675347328186,
-0.4136529564857483,
-0.19969521462917328,
0.24256658554077148,
-0.49622243642807007,
-0.24250133335590363,
0.24068671464920044,
-0.22222016751766205,
-0.499637246131897,
-0.5957363247871399,
-0.282170832157135,
0.4913678467273712,
0.406749963760376,
-0.756505012512207,
0.4657745063304901,
-0.08925586193799973,
0.06562135368585587,
-0.507696807384491,
-0.4016004502773285,
-0.0952700600028038,
0.21311083436012268,
-0.3855665922164917,
0.10270549356937408,
0.026606695726513863,
-0.09138842672109604,
0.11841700971126556,
-0.4642561376094818,
0.025184210389852524,
0.004731615539640188,
0.5844969153404236,
0.42865556478500366,
-0.13601475954055786,
-0.05495994910597801,
0.05785733461380005,
0.5821405053138733,
-0.06729748100042343,
-0.35919663310050964,
0.3233095705509186,
0.0783618614077568,
-0.08898073434829712,
0.3933505415916443,
0.45335716009140015,
0.520857572555542,
-0.06594058126211166,
-0.599298357963562,
0.4990916848182678,
0.9539217352867126,
-0.5498716235160828,
0.6242968440055847,
0.4068309962749481,
-0.6890344619750977,
-0.4730125367641449,
-0.036510057747364044,
-0.055156901478767395,
0.5930131673812866,
0.16974514722824097,
-0.29313650727272034,
-0.20062747597694397,
-0.25148141384124756,
0.3728916049003601,
0.5245606899261475,
0.2450956553220749,
0.03806658089160919,
-0.10370144248008728,
-0.4712374210357666,
0.20802931487560272,
-0.3206435441970825,
-0.020293334499001503,
0.5362504124641418,
0.5802887678146362,
0.06200878322124481,
-0.4358827471733093,
0.06968789547681808,
-0.29708442091941833,
0.08046449720859528,
0.6437464356422424,
-0.01155330054461956,
0.5912192463874817,
0.08416901528835297,
0.06920186430215836,
-0.27845537662506104,
0.3545229136943817,
1.2567505836486816,
-0.4521578550338745,
-0.4411540627479553,
-0.00291455234400928,
0.5818383693695068,
-0.30328893661499023,
0.6115019917488098,
0.47303688526153564,
-0.07074106484651566,
0.05804378539323807,
0.00649519357830286,
-0.09021381288766861,
-0.23881582915782928,
-0.059289656579494476,
-0.5543837547302246,
0.3486168682575226,
0.3365457355976105,
-0.3481726050376892,
0.17612433433532715,
0.22342054545879364,
0.40870726108551025,
-0.3880607783794403,
-0.7240088582038879,
0.23433144390583038,
-0.5798696279525757,
0.15251260995864868,
-0.2672197222709656,
-0.41193777322769165,
0.2691083252429962,
0.37673041224479675,
-0.19260837137699127,
0.0035875483881682158,
-0.01553330197930336,
-0.04948608577251434,
-0.055649805814027786,
0.13774226605892181,
0.1729011982679367,
0.12679848074913025,
0.4185743033885956,
-1.1096819639205933,
0.19310341775417328,
-0.13773569464683533,
0.24868826568126678,
-0.308489590883255,
0.10300196707248688,
-0.04956793040037155,
-0.1292261779308319,
-0.8170287609100342,
-0.2858811914920807,
0.5542563796043396,
-0.24516816437244415,
-0.5970034599304199,
-0.025739425793290138,
0.3152119815349579,
-0.41939184069633484,
0.28163039684295654,
-0.7392376065254211,
0.9387938380241394,
-0.2908463776111603,
0.20375776290893555,
-0.3144810199737549,
0.03426680341362953,
0.7681645154953003,
-0.5857085585594177,
-0.38357704877853394,
-0.6529456377029419,
-0.6186540126800537,
0.5118719935417175,
0.6420303583145142,
0.0016001989133656025,
-0.5553589463233948,
0.08392469584941864,
-0.13142874836921692,
-0.2032153457403183,
0.17194829881191254,
-0.2054905891418457,
0.5391964316368103,
-0.17809046804904938,
-0.06667160987854004,
-0.8393707275390625,
-0.2201581448316574,
-0.1942593902349472,
0.18177016079425812,
-0.4977770447731018,
-0.6884317398071289,
0.7184789776802063,
-0.21818087995052338,
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] |
Deposition
technique
used
Thickness
(nm)
Substrate used
Average optical
Transmittance
(%)
Optical
band
gap
(eV)
Electrical
conductivity
(S/cm)
Carrier
conc
(/cm3)
Hall
Mobility
(cm2/V-s)
Reference
NiO
Magnetron
Sputtering
110
glass
40
3.8
7.2
1.3×1019
-
[5]
NiO
RFMS
100
glass
69
-
9.09
8.8×1018
6.12
[96]
K:NiO
PLD
100
glass
60
3.73-
3.88
4.25
7.18×1019
0.37
[97]
Cu-NiO
Reactive
Sputtering
500
Silicon
-
2.41
8.34
4.22×1020
1
[98]
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] |
[97]
Cu-NiO
Reactive
Sputtering
500
Silicon
-
2.41
8.34
4.22×1020
1
[98]
SnxNiyOz
RFMS
100
InP
-
2.9
0.071
2.04×1017
7.7
[101]
Mn:NiO
spray
pyrolysis
200
glass
84
3.61
1.19
-
-
[102]
Zn:NiO
spray
pyrolysis
200
glass
73
3.67
3.79
-
-
[102]
ZnO
PLD
700-1400
Fused Silica
80
-
0.5
5.6×1018
0.1
[107]
SnO
PLD
110
YSZ
-
2.7
-
2.5×1017
2.4
[121]
SnOx
RFMS
200
glass
85
2.8
0.1-0.01
1017-1018
4.8
[123]
SnO
RFMS
200-300
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] |
RFMS
200
glass
85
2.8
0.1-0.01
1017-1018
4.8
[123]
SnO
RFMS
200-300
Soda lime glass
57
2.7-2.9
1.16
45.7×1017
1.6
[124]
Ga-SnO
RFMS
200-300
Soda lime glass
65
2.7-2.9
3.71
62.4×1017
3.6
[124]
Na-SnO
RFMS
200-300
Soda lime glass
50
2.7-2.9
90.9
469×1017
11.3
[124]
Ga:SnO2
DC
magnetron
sputtering
200
Quartz
85
3.8
0.021
8.84×1018
0.0146
[129]
Eu-doped
SnO2
spray
pyrolysis
700
Si (100) and
glass
70-80
3.68-
3.73
0.02-0.06
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0.20069845020771027,
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0.306753545999527,
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0.2545813322067261,
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0.04108876734972,
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] |
SnO2
spray
pyrolysis
700
Si (100) and
glass
70-80
3.68-
3.73
0.02-0.06
9.12×1019
57.1-2.71
[130]
Cu2O
PLD
100
MgO
-
-
-
1020
90
[140]
Cu2O
Thermal
Evaporation
223
ITO and glass
-
2.0
2.74×10-3
2.8×1015
6.1
[142]
Table 5: Chalcogen-based materials as p-type TCO and their respective optoelectronic parameters.
Material
Deposition
technique
used
Thickness
(nm)
Substrate used
Average optical
Transmittance
(%)
Optical
band
gap
(eV)
Electrical
conductivity | [
0.2830505967140198,
0.034293439239263535,
0.4985405504703522,
0.08445703983306885,
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0.10928947478532791,
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-0.062343548983335495,
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0.5161524415016174,
0.013069162145256996,
-0.08778628706932068,
0.20527684688568115,
0.4849812686443329,
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] |
Average optical
Transmittance
(%)
Optical
band
gap
(eV)
Electrical
conductivity
(S/cm)
Carrier
conc
(/cm3)
Hall
Mobility
(cm2/V-s)
Reference
La1-xSrxCuOS
RF
Sputtering
130
Silica glass
>70
3.1
0.26
-
-
[53]
LaCuOS1-x Sex
Reactive
Solid phase
150
MgO
-
-
24
⁓1018
8
[54]
Mg-LaCuOSe
Reactive
Solid phase
40
MgO
70
2.8
140
2.2×1020
3.5
[56]
(La1-xSrxO)CuS
RF
Sputtering
150
SiO2
>60
-
20
-
-
[56]
La1−xYxCuOS
Spin coating
250
Quartz
⁓70
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-0.4555072784423828,
-0.34354349970817566,
0.1853857785463333,
-0.3409915566444397,
0.12262238562107086,
-0.2495071142911911,
-0.2615073323249817,
0.40373116731643677,
0.33154723048210144,
-0.42522120475769043,
0.18022684752941132,
0.2796151638031006,
0.19663436710834503,
0.02342505007982254,
0.13365742564201355,
0.3903718590736389,
-0.336076021194458,
0.24218197166919708,
-1.1767977476119995,
-0.22147029638290405,
0.16982059180736542,
0.1803988814353943,
-0.10333049297332764,
0.3029268980026245,
-0.32389265298843384,
-0.26682597398757935,
-0.3940565586090088,
0.1108880415558815,
0.7003732919692993,
-0.6952905058860779,
-0.6767008900642395,
0.02671133540570736,
0.35436397790908813,
-0.3825884759426117,
0.216147780418396,
-0.13443942368030548,
0.8311218619346619,
-0.015352257527410984,
-0.21262218058109283,
-0.7124657034873962,
-0.13638386130332947,
1.0293452739715576,
-0.6207022070884705,
-0.08725294470787048,
-0.33449116349220276,
-0.3732060492038727,
-0.1425127238035202,
0.36882561445236206,
-0.042978230863809586,
-0.8290728330612183,
0.42401817440986633,
0.1712273210287094,
0.11211282759904861,
-0.05241701751947403,
0.37602052092552185,
0.6397728323936462,
-0.6651275753974915,
0.05255692079663277,
-0.7112098336219788,
0.3030277490615845,
-0.20362581312656403,
0.03081420809030533,
-0.6499530076980591,
-0.6457823514938354,
0.2989605963230133,
0.04798935726284981,
0.1426863968372345,
0.13813838362693787,
-0.11429473012685776,
0.17635253071784973,
-0.7792931199073792,
0.14269565045833588,
0.2952860891819,
0.06444994360208511,
-1.0060150623321533,
-0.18084384500980377,
0.06220518425107002,
0.716890811920166,
0.0612022802233696,
0.2687559127807617,
-0.17391347885131836,
0.13810847699642181,
-0.36476534605026245,
0.2900661528110504,
0.6945438385009766,
-0.7436904907226562,
0.21044081449508667,
-0.4030928611755371,
0.15527532994747162,
-0.14380279183387756,
0.032693348824977875,
-0.26979753375053406,
0.1797861009836197,
0.06740493327379227,
-0.0214497409760952,
0.4717554450035095,
-0.3297535479068756,
-0.13930337131023407,
0.04151709005236626,
0.32623228430747986,
0.16056503355503082,
0.3553606867790222,
-0.06580324470996857,
0.939742386341095,
0.4401319622993469,
0.050142690539360046,
-0.3658497631549835,
0.7444697022438049,
-0.2807938754558563,
-0.08757953345775604,
0.16537517309188843,
0.3745613098144531,
0.38645705580711365,
-0.25615134835243225,
-0.24727603793144226,
0.3732878565788269,
0.249977245926857,
0.014338466338813305,
-0.23358264565467834,
-0.451133668422699,
-0.2919650971889496,
0.29535970091819763,
0.5017750859260559,
0.6187231540679932,
-0.3713151216506958,
-0.004752760287374258,
0.06021875515580177,
0.2427452653646469,
-0.1616574227809906,
-0.4529896378517151,
0.06946267932653427,
0.17119291424751282,
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-0.2463882714509964,
-0.20944514870643616,
-0.3146502375602722,
-0.7432138919830322,
0.054003309458494186,
-0.19480538368225098,
0.04950207099318504,
-0.736666202545166,
-0.02856084704399109,
-0.18852181732654572,
0.11033210158348083,
-0.19362720847129822,
-0.0879325196146965,
-0.9243321418762207,
-0.514603316783905,
0.06430631875991821,
0.3944479525089264,
-0.40196895599365234,
-0.42134737968444824,
-0.0708196610212326,
0.04783777892589569,
0.05252417176961899,
0.7083592414855957,
0.08009769022464752,
-0.681826651096344,
0.18681691586971283,
0.09964845329523087,
0.15011066198349,
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0.4987356662750244,
-0.30617955327033997,
-0.7071090340614319,
-0.21384426951408386,
-0.09276210516691208,
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0.23016780614852905,
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0.6192433834075928,
-0.21003733575344086,
-0.19203920662403107,
-0.040659040212631226,
-0.3730526566505432,
-0.4508792459964752,
-0.02129301428794861,
0.6857487559318542,
0.42443907260894775,
0.2730729877948761,
-0.08748610317707062,
-0.03673389181494713,
0.021057654172182083,
0.7306424975395203,
-0.6136763095855713,
0.4541114866733551,
-0.5003353357315063,
0.31453123688697815,
-0.5840252041816711,
-0.1970692127943039,
0.6786196231842041,
0.04495205357670784,
-0.174122154712677,
0.09531567990779877,
0.13518093526363373,
0.04368945583701134,
0.4996175765991211,
-0.5145201086997986,
-0.3791346848011017,
-0.29710331559181213,
-0.34913370013237,
-0.5314624905586243,
0.8714726567268372,
0.13943703472614288,
0.4546297490596771,
0.25739043951034546,
0.28499525785446167,
0.1385345160961151,
0.5937528610229492,
0.3340442180633545,
-0.0028318141121417284,
-0.02475121058523655,
-0.04984866455197334,
0.6628704071044922,
-0.33202484250068665,
0.21773101389408112,
-0.1769833117723465,
0.2779998481273651,
-0.20904536545276642,
0.0009747903677634895,
-0.13753212988376617,
-1.0443463325500488,
-0.41905829310417175,
-0.07205493003129959,
-0.056904565542936325,
0.11423631012439728,
-0.010542569682002068,
-0.39514636993408203,
-0.5796723961830139,
0.271200567483902,
-0.11475683748722076,
-0.6504113674163818,
0.070619136095047,
0.0026270777452737093,
-0.02882254682481289,
-0.282335102558136,
-0.15379753708839417,
-0.15183408558368683,
-0.009158710017800331,
-0.313603937625885
] |
RF
Sputtering
150
SiO2
>60
-
20
-
-
[56]
La1−xYxCuOS
Spin coating
250
Quartz
⁓70
3
89.3
6.6×1020
0.85
[147]
La1-xSrxCuOS
RF
Sputtering
130
Silica glass
>70
3.1
0.26
-
-
[53]
Table 6: Cr-based materials as p-type TCO and their respective optoelectronic parameters.
Material
Deposition
technique
used
Thickness
(nm)
Substrate
used
Average optical
Transmittance
(%)
Optical
band gap
(eV)
Electrical
conductivity
(S/cm)
Carrier
conc
(/cm3)
Hall
Mobility | [
0.08652079850435257,
0.2505582869052887,
0.9819210171699524,
0.09121080487966537,
-0.36283496022224426,
-0.07650677114725113,
0.08175063878297806,
-0.8997204303741455,
-0.1567625254392624,
0.1131826788187027,
-0.20095455646514893,
0.6401429772377014,
-0.026303473860025406,
0.03572097420692444,
0.2099715769290924,
0.9814057946205139,
0.768132746219635,
0.47021278738975525,
-0.07562166452407837,
-1.0300041437149048,
0.17697852849960327,
-0.18965265154838562,
0.8314343690872192,
-0.18098688125610352,
0.19538378715515137,
0.37234529852867126,
0.17112702131271362,
0.19588151574134827,
0.18864023685455322,
0.21938729286193848,
0.07979979366064072,
0.8820207715034485,
-0.024996351450681686,
-0.013768255710601807,
0.6896259784698486,
0.3741702139377594,
0.059966858476400375,
-0.22091059386730194,
-0.07833544909954071,
-0.5959584712982178,
0.17473207414150238,
-0.19392229616641998,
-0.24643567204475403,
0.46971395611763,
-0.030684292316436768,
-0.15461157262325287,
-1.1175004243850708,
0.4365841746330261,
-0.30535659193992615,
0.14583519101142883,
0.10365607589483261,
0.32261115312576294,
0.12504512071609497,
0.19348746538162231,
0.08440275490283966,
0.17576633393764496,
-0.7091726064682007,
-0.15092843770980835,
0.5517146587371826,
-0.18057845532894135,
0.3114495575428009,
-0.10517449676990509,
-0.6664232611656189,
0.4376131296157837,
0.05201747268438339,
0.5334832668304443,
0.06838097423315048,
-0.032043784856796265,
-0.15002748370170593,
0.37335124611854553,
0.9079768061637878,
-0.07622186839580536,
0.1849675476551056,
0.09145230799913406,
-0.09236390888690948,
0.18051087856292725,
-0.0752253457903862,
-0.007801661267876625,
0.05240054428577423,
0.316448450088501,
0.38222160935401917,
0.00770486518740654,
0.5619072318077087,
0.07306148111820221,
0.408243328332901,
-0.20166821777820587,
-0.09613896906375885,
0.6514630913734436,
-0.5424285531044006,
0.3169800639152527,
-0.03075498342514038,
-0.26234811544418335,
0.3434656262397766,
0.42845264077186584,
0.09282101690769196,
-0.10649079829454422,
-0.38205501437187195,
-0.15376578271389008,
0.3123812973499298,
0.08228734880685806,
-0.11073752492666245,
0.22226044535636902,
-0.149826318025589,
-0.09498285502195358,
-0.1552952229976654,
-0.27976593375205994,
-0.8115918040275574,
-0.7900994420051575,
-0.2872362434864044,
-0.011024818755686283,
-0.5475794076919556,
-0.19719310104846954,
-0.22138239443302155,
-0.20039816200733185,
-0.401867538690567,
0.049162812530994415,
0.23217074573040009,
0.13773944973945618,
0.33905234932899475,
0.5542604327201843,
-0.11277899891138077,
1.026654601097107,
-0.1945648342370987,
0.22794656455516815,
0.44090667366981506,
0.06723495572805405,
0.8747819662094116,
0.697960376739502,
-0.5471200346946716,
0.6062082648277283,
0.0006940391613170505,
1.183292031288147,
-0.19757844507694244,
-0.09198654443025589,
-0.006871647667139769,
-0.6646146178245544,
-0.17145982384681702,
0.039328042417764664,
0.15287752449512482,
0.348081111907959,
-0.3635537028312683,
-0.6000264286994934,
-0.3355324864387512,
0.0936368852853775,
-0.3286686837673187,
-0.27997204661369324,
-0.43384402990341187,
-0.1194033995270729,
-0.8126709461212158,
0.015036766417324543,
-0.11974966526031494,
-0.08006628602743149,
-0.20130346715450287,
0.007317493669688702,
-0.08349106460809708,
0.3199214041233063,
0.35581088066101074,
-0.03847414255142212,
-0.5719998478889465,
0.014716600999236107,
0.20124629139900208,
-0.13403479754924774,
-0.5393739342689514,
0.10724406689405441,
0.6528915762901306,
0.1080273911356926,
0.10064056515693665,
0.0667608454823494,
-0.03381770849227905,
0.3049313426017761,
-0.018667085096240044,
-0.11429324001073837,
-0.14727932214736938,
-0.14797140657901764,
0.21804498136043549,
0.2780701816082001,
0.24902687966823578,
0.13177573680877686,
-0.16145853698253632,
0.43019965291023254,
-0.5729058384895325,
-0.1598779261112213,
-0.004363119602203369,
-0.3051706552505493,
0.32961320877075195,
0.5251345634460449,
0.9083738327026367,
0.24011510610580444,
0.09848175197839737,
0.14022484421730042,
-0.2886163592338562,
-0.1725754290819168,
0.7432337999343872,
-0.6790525913238525,
1.5681788921356201,
0.23358502984046936,
0.0036174324341118336,
0.37306833267211914,
0.25787001848220825,
0.1576930731534958,
-0.17309774458408356,
0.3780520558357239,
0.5684337019920349,
-0.4403264820575714,
-0.708417534828186,
0.11187286674976349,
0.19513382017612457,
-0.212124302983284,
-0.16484245657920837,
-0.17188793420791626,
0.545483410358429,
-0.6559270620346069,
-0.5146900415420532,
-0.4530419111251831,
0.1035018265247345,
-0.5400816202163696,
-0.09143184125423431,
0.09532015025615692,
0.37270838022232056,
-0.09783343970775604,
0.6010714173316956,
-0.5256800055503845,
0.336494117975235,
0.829939603805542,
-0.5938762426376343,
0.8245741128921509,
0.3704962134361267,
-0.14260169863700867,
0.508241593837738,
-0.5326237678527832,
0.26781994104385376,
-0.2525974214076996,
0.4056941568851471,
-0.3187437653541565,
-0.019505778327584267,
-0.05274437740445137,
0.16396568715572357,
0.10685714334249496,
0.6146752834320068,
-0.31222155690193176,
0.017992621287703514,
0.6798635125160217,
-0.5102983117103577,
-0.03108232095837593,
0.018746094778180122,
-0.3885686993598938,
0.02406574785709381,
-0.021347317844629288,
-0.18629904091358185,
0.0007093983003869653,
0.285213440656662,
0.3946015536785126,
-0.21584771573543549,
-0.9985958933830261,
-0.11999846249818802,
-0.22159145772457123,
0.15454363822937012,
-0.25020039081573486,
-0.3121016025543213,
-0.4854854345321655,
-0.7455949783325195,
-0.28904613852500916,
0.16137555241584778,
-0.18717126548290253,
-0.08364425599575043,
-0.4419674277305603,
-0.439644455909729,
-0.5004698038101196,
0.837573766708374,
0.4173101782798767,
-0.19186931848526,
0.1048177108168602,
-0.37987205386161804,
-0.010039466433227062,
-0.14934474229812622,
-0.5337491035461426,
0.3827044367790222,
0.32748645544052124,
-0.617298424243927,
-0.559662401676178,
0.05365925654768944,
0.6123372316360474,
1.3012101650238037,
-0.2341606616973877,
-0.768095076084137,
0.336656391620636,
-0.14435823261737823,
0.0743633508682251,
-0.5750311017036438,
-0.7622798085212708,
-0.5855088233947754,
0.5032901167869568,
0.05328378081321716,
-0.2611238658428192,
-0.09061119705438614,
0.6410510540008545,
-0.015718139708042145,
0.4946630299091339,
0.6976195573806763,
-0.16108672320842743,
-0.38714155554771423,
-0.20466861128807068,
-0.6217626333236694,
0.1316232979297638,
-0.16117270290851593,
-0.4788813889026642,
-0.6284531950950623,
0.13775935769081116,
-5.726604461669922,
0.04702240601181984,
-0.3434562385082245,
0.046899911016225815,
-0.3820894658565521,
0.16150832176208496,
0.8215530514717102,
-0.04334729164838791,
0.1968364119529724,
0.008418722078204155,
0.041891805827617645,
0.7047473788261414,
0.22663642466068268,
0.0058592138811945915,
0.33879074454307556,
0.3989832103252411,
0.3510819375514984,
-0.3225288391113281,
0.28029048442840576,
-0.21567705273628235,
0.40226176381111145,
0.2791353762149811,
0.00024247249530162662,
0.03207191824913025,
0.0949888601899147,
0.12035398185253143,
-1.1091721057891846,
0.4112040400505066,
-0.35259395837783813,
-0.36562874913215637,
0.17626763880252838,
-0.44725891947746277,
-0.28568679094314575,
-0.17067402601242065,
0.03341980651021004,
-0.0620887465775013,
0.6576396226882935,
0.032647304236888885,
-0.6063020825386047,
-0.11374079436063766,
0.7362435460090637,
0.055333517491817474,
-0.11420589685440063,
-0.04344696179032326,
0.6418069005012512,
-0.2333238571882248,
-0.22535854578018188,
0.024511484429240227,
0.08777032792568207,
0.5765362977981567,
-0.10070588439702988,
-0.5260494351387024,
0.05724585801362991,
0.15448510646820068,
0.27100279927253723,
0.08580749481916428,
0.12468308210372925,
0.50444096326828,
-0.5358787178993225,
-0.06135687232017517,
-0.6245853900909424,
-0.17743204534053802,
-0.24098291993141174,
-0.5954149961471558,
-0.5129575133323669,
0.8369866609573364,
-0.8572920560836792,
-0.4691014289855957,
0.6370999813079834,
-0.15370231866836548,
-0.22624537348747253,
0.38997337222099304,
-0.04503763094544411,
-0.4920065402984619,
0.5334280729293823,
-0.4182952046394348,
0.7184610366821289,
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] |
Optical
band gap
(eV)
Electrical
conductivity
(S/cm)
Carrier
conc
(/cm3)
Hall
Mobility
(cm2/V-s)
FOM
(μS)
Reference
Mg,N:Cr2O3
Spray
pyrolysis
150
Glass
10-65
3.1
0.06
1019
0.1
7.2
[152]
Ni:Cr2O3
PLD
150
Sapphire
40
-
28
-
-
110
[154]
Cr2O3
PLD
75
Sapphire
80
3.64
0.008
1.93×1018
0.1
0.29
[155]
Mg:Cr2O3
PLD
75
Sapphire
70
3.54
0.4
2.04×1018
0.4
8.16
[155]
Al:Cr2O3
PLD
75
Sapphire
81
3.59
0.009
1.90×1018
0.11
0.33
[155]
Ni:Cr2O3
PLD | [
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0.23670437932014465,
0.1800820380449295,
-0.2543199062347412,
0.184566929936409,
-0.04501926526427269,
-0.15500600636005402,
-0.2606464922428131,
0.26348474621772766,
-0.20859597623348236,
-0.08339923620223999,
-0.4423733949661255,
0.01646069623529911,
-0.3249300420284271,
0.3912927806377411,
-0.3949134349822998,
-0.16638965904712677,
-0.11291780322790146,
-0.31696730852127075,
-0.179620161652565,
0.6539811491966248,
-0.45167437195777893,
-0.15210847556591034,
-0.2791030704975128,
-0.6229986548423767,
-0.17427761852741241,
0.525844395160675,
-0.31605038046836853,
-0.20497183501720428,
0.36136671900749207,
-0.6548526883125305,
-0.058782681822776794,
-0.17384473979473114,
-0.1982528269290924,
0.2378372699022293,
0.4969112277030945,
-0.5784543752670288,
-0.33786049485206604,
0.4100164771080017,
0.31833818554878235,
0.9086233973503113,
0.07878376543521881,
-0.7111340761184692,
-0.5880645513534546,
0.054932851344347,
-0.5302449464797974,
-0.9976004958152771,
-0.8871017694473267,
-0.0897054597735405,
0.8949029445648193,
0.06246205419301987,
-0.23603489995002747,
0.10526338219642639,
0.40160566568374634,
-0.2909299433231354,
0.08264843374490738,
0.6491395831108093,
-0.24332483112812042,
0.323283851146698,
-0.03786608576774597,
-0.4755435585975647,
0.3098764717578888,
0.030928967520594597,
-0.7692679166793823,
-0.16823332011699677,
-0.07163979113101959,
-5.43213415145874,
0.3622952401638031,
-0.3995034396648407,
0.3758731782436371,
-0.6818566918373108,
-0.049375537782907486,
1.0913031101226807,
-0.16388830542564392,
0.5658712983131409,
-0.17578409612178802,
-0.051565688103437424,
0.3191806674003601,
0.015119885094463825,
0.01354540791362524,
0.5549969673156738,
0.9541807770729065,
0.3487229645252228,
-0.25961437821388245,
0.5930300354957581,
-0.07336645573377609,
0.624180257320404,
-0.12247341126203537,
-0.44320377707481384,
0.12756142020225525,
0.418328195810318,
-0.6506820917129517,
-0.5481064319610596,
0.1275683045387268,
0.035920191556215286,
-0.14116080105304718,
0.45551109313964844,
-0.38720789551734924,
-0.3415701687335968,
-0.22350922226905823,
0.22237782180309296,
-0.01765494793653488,
0.8957601189613342,
-0.058798592537641525,
-0.2728458642959595,
-0.8338164687156677,
0.8722248077392578,
1.0833607912063599,
0.3710077702999115,
0.31030136346817017,
0.7626205682754517,
0.16207395493984222,
-0.024293988943099976,
0.014385598711669445,
0.15419073402881622,
0.8316466212272644,
-0.22300474345684052,
-0.27671441435813904,
0.149287149310112,
-0.016842173412442207,
-0.0818149596452713,
0.17680512368679047,
-0.44690820574760437,
0.7612916827201843,
-0.4162547290325165,
0.2810226082801819,
-0.27969348430633545,
-0.044967181980609894,
-0.3616101145744324,
-0.5167515873908997,
-0.4255761504173279,
0.32198524475097656,
-1.086976170539856,
-0.18875880539417267,
0.40496626496315,
-0.2055509388446808,
-0.7246654629707336,
0.5139315724372864,
-0.30742859840393066,
-0.5146246552467346,
0.3190741240978241,
-0.01739700883626938,
1.0428088903427124,
-0.028723541647195816,
-0.7756642699241638,
0.5223810076713562,
-0.3929418921470642,
-0.52269446849823,
0.2157692313194275,
0.6887103319168091,
-0.024148941040039062,
-0.3745926320552826,
-0.09856060892343521,
-0.10437247902154922,
-0.2700986862182617,
0.02206479199230671,
0.5704663395881653,
-0.03509709984064102,
0.08112149685621262,
-0.046541109681129456,
0.30408257246017456,
-0.2905927002429962,
0.4311618208885193,
0.444532185792923,
0.5519104599952698,
0.1764378696680069,
0.32777050137519836,
-0.017287936061620712,
0.21259814500808716,
-0.9699311852455139,
-0.6567833423614502,
0.3477841913700104,
-0.421311616897583,
-0.1823401004076004,
0.44706839323043823,
-0.11061175912618637,
0.3464006185531616,
-0.16482098400592804,
-0.6063244938850403,
0.37382781505584717,
0.9112151861190796,
-0.6838493943214417,
0.17744362354278564,
0.12669752538204193,
0.0625426173210144,
-0.4836488664150238,
-0.3739560544490814,
0.35258227586746216,
0.040651604533195496,
-0.15522810816764832,
-0.723396360874176,
-0.36315110325813293,
-0.1976339966058731,
0.7612863183021545,
-0.6111138463020325,
0.3601222038269043,
0.2948574423789978,
0.6595542430877686,
-0.3646189570426941,
-0.22891166806221008,
-0.18083900213241577,
-0.6015852093696594,
-0.45181167125701904,
0.34369534254074097,
0.38257327675819397,
-0.13735456764698029,
0.5249403715133667,
-0.5407152771949768,
-0.16918280720710754,
-0.21691450476646423,
0.22639669477939606,
0.466988205909729,
-0.3361530601978302,
0.21909360587596893,
-0.4121705889701843,
0.36005881428718567,
-0.10728557407855988,
-0.47575077414512634,
0.2498098760843277,
0.030138880014419556,
0.248066246509552,
0.23938259482383728,
0.06799433380365372,
-0.12087444216012955,
0.1453382819890976,
-0.8371182680130005,
0.481268048286438,
1.037528395652771,
-0.7616596221923828,
0.2480388730764389,
0.18619172275066376,
-0.32970166206359863,
-0.7198385000228882,
-0.24749861657619476,
0.13057169318199158,
0.40121540427207947,
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0.6322786808013916,
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-0.6690106391906738,
0.47930052876472473,
0.15373937785625458,
-0.17456303536891937,
0.6965667605400085,
0.4700244665145874,
-0.15452003479003906,
-0.28937748074531555,
-0.06716206669807434,
-0.18881173431873322,
-0.05156709626317024,
0.5399436950683594,
0.027644691988825798,
0.24418193101882935,
-0.41472193598747253,
0.0392424501478672,
-0.4380257725715637,
0.2954610288143158,
1.0856877565383911,
-0.3653320372104645,
-0.6335105299949646,
-0.07804198563098907,
0.20741930603981018,
-0.5412411689758301,
0.6608191132545471,
-0.12150566279888153,
0.12665781378746033,
0.13640086352825165,
0.19234924018383026,
-0.5049086213111877,
-0.2727571725845337,
-0.5547522902488708,
-0.6627499461174011,
-0.41960424184799194,
0.4245075583457947,
-0.10555827617645264,
0.29874828457832336,
-0.11175157129764557,
0.22094982862472534,
-0.3965498208999634,
-0.6079596281051636,
0.2082596868276596,
-0.688238263130188,
0.3412383496761322,
-0.005495763383805752,
-0.495714008808136,
0.6978729367256165,
0.12241190671920776,
-0.18556062877178192,
0.22270238399505615,
0.2173917442560196,
-0.6406443119049072,
-0.04466328024864197,
0.10292813181877136,
0.49902433156967163,
-0.18202106654644012,
0.21237127482891083,
-1.3057143688201904,
-0.16470004618167877,
0.03757096081972122,
0.5865983366966248,
-0.22531506419181824,
-0.02026507444679737,
-0.6413090229034424,
-0.2659611105918884,
-0.7496473789215088,
0.16241669654846191,
0.568449854850769,
-0.41736748814582825,
-0.5758209228515625,
0.13086360692977905,
-0.07688415050506592,
-0.547675609588623,
0.0017116948729380965,
-0.3766103684902191,
1.025771975517273,
0.045223839581012726,
-0.21765512228012085,
-0.4786808490753174,
-0.33632317185401917,
0.9005945324897766,
-0.6947561502456665,
-0.36570268869400024,
-0.6112723350524902,
-0.4675314426422119,
0.3584108054637909,
0.5393027067184448,
-0.13463377952575684,
-1.2189342975616455,
0.3112814128398895,
-0.002654475625604391,
0.15855003893375397,
-0.19063614308834076,
0.7898579239845276,
0.6830894947052002,
-0.6965197920799255,
0.3406001329421997,
-0.6242659091949463,
0.12846413254737854,
-0.3107115924358368,
-0.05409780517220497,
-0.5818696022033691,
-0.5891833305358887,
0.3939235508441925,
-0.06510169059038162,
0.29322850704193115,
0.17133091390132904,
0.014594404958188534,
-0.10714177042245865,
-0.5643924474716187,
0.24364714324474335,
0.3002607524394989,
-0.08877463638782501,
-1.1395317316055298,
-0.13377615809440613,
0.03519038110971451,
0.5900550484657288,
0.20827345550060272,
0.06954742223024368,
-0.09228433668613434,
-0.04207472503185272,
-0.3161551356315613,
0.2617718577384949,
0.5402241349220276,
-0.7850437760353088,
0.31271952390670776,
-0.25738784670829773,
0.08868348598480225,
0.06972534954547882,
-0.024296754971146584,
-0.26819005608558655,
0.04841984435915947,
-0.03654435649514198,
0.0377984493970871,
0.7021164894104004,
-0.28465697169303894,
-0.08301349729299545,
0.5964944958686829,
0.23485954105854034,
-0.10677476227283478,
0.18929395079612732,
-0.044579461216926575,
0.6848825812339783,
0.4295252859592438,
0.23313197493553162,
-0.8209274411201477,
0.4799708127975464,
-0.009838292375206947,
-0.29064300656318665,
0.1753988116979599,
0.3603041470050812,
0.5627616047859192,
-0.10980074107646942,
-0.07594086974859238,
0.6364520192146301,
0.502310037612915,
-0.040448933839797974,
-0.29529884457588196,
-0.4074166715145111,
-0.2548597753047943,
0.483003169298172,
0.18761932849884033,
0.8589601516723633,
-0.24918672442436218,
0.35206979513168335,
-0.17356106638908386,
0.3929564952850342,
0.05106573924422264,
-0.1564197689294815,
-0.21433252096176147,
0.3442683517932892,
-0.38425174355506897,
-0.4593330919742584,
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-0.6731030344963074,
-1.0509517192840576,
0.2270323932170868,
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0.04758533835411072,
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0.019465966150164604,
-0.09366219490766525,
0.19536830484867096,
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-0.49600502848625183,
0.30506670475006104,
0.2359701544046402,
0.21872444450855255,
0.7466551661491394,
-0.17179247736930847,
-0.37795448303222656,
0.35712727904319763,
0.01223687268793583,
0.010163663886487484,
0.1929934322834015,
-0.46508434414863586,
0.5451701879501343,
-0.1280605047941208,
-1.0132561922073364,
0.043473660945892334,
-0.1484021544456482,
0.2169026881456375,
0.649391233921051,
0.13688966631889343,
-0.5631078481674194,
0.6416725516319275,
-0.28195124864578247,
0.16471531987190247,
-0.17645615339279175,
-0.14808912575244904,
-0.6274486184120178,
0.1269119679927826,
0.5148345828056335,
0.5699025392532349,
0.34482714533805847,
0.22805261611938477,
0.02182706445455551,
0.23559501767158508,
0.4296499192714691,
-0.5004815459251404,
0.817920446395874,
-0.4130484163761139,
0.3623337149620056,
-0.7238818407058716,
-0.4256923794746399,
1.0987203121185303,
-0.3444051444530487,
0.07751352339982986,
0.003941838629543781,
-0.10190874338150024,
-0.028828518465161324,
0.8060778379440308,
-0.3790331780910492,
-0.37624678015708923,
-0.5935764312744141,
-0.45231252908706665,
-0.88423091173172,
0.34643682837486267,
0.03157206252217293,
0.4420718252658844,
0.2309153825044632,
0.8093820214271545,
0.15408898890018463,
0.670907735824585,
0.2696572244167328,
0.2315024584531784,
-0.3935532867908478,
-0.26815682649612427,
0.854594349861145,
-0.4363726079463959,
0.19134804606437683,
-0.2936091721057892,
0.4850519597530365,
-0.35609567165374756,
-0.0056991553865373135,
-0.6084797978401184,
-0.6672778129577637,
-0.4936663508415222,
0.19667911529541016,
-0.09963709115982056,
0.26370763778686523,
-0.14324761927127838,
-0.8495946526527405,
-0.99303138256073,
0.16128206253051758,
0.30148252844810486,
-0.898827314376831,
0.1183258518576622,
0.059228360652923584,
-0.2819784879684448,
-0.16981512308120728,
-0.014836601912975311,
0.00021107295469846576,
-0.15211538970470428,
-0.19761566817760468
] |
[155]
Al:Cr2O3
PLD
75
Sapphire
81
3.59
0.009
1.90×1018
0.11
0.33
[155]
Ni:Cr2O3
PLD
75
Sapphire
78
3.49
1.17
7.24×1018
2
34.62
[156]
Sr-LaCrO3
MBE
50
STO
42.3
1.9
54
7.5×1021
0.04
3050
[158]
La0.75Sr0.25CrO3
Spin
coating
45
STO and
LAO
67
-
1
-
-
-
[159]
Mg,N:Cr2O3
Spray
pyrolysis
150
Glass
10-65
3.1
0.06
1019
0.1
7.2
[152]
Table 7: Some other oxide materials as p-type TCO and their respective optoelectronic parameters.
Material
Deposition | [
0.2557890713214874,
0.40631312131881714,
0.24457208812236786,
0.0455472432076931,
-0.2376529723405838,
0.3142673373222351,
0.3532364070415497,
-0.6211466789245605,
-0.1269310712814331,
0.07631540298461914,
-0.1862637847661972,
0.6838115453720093,
-0.06995297968387604,
0.2565326392650604,
0.34890982508659363,
1.2057628631591797,
0.7278311252593994,
0.5211210250854492,
0.1652156412601471,
-0.8087247014045715,
0.12322486937046051,
-0.3275640606880188,
0.9232578873634338,
-0.186392143368721,
0.2124410718679428,
0.6119266748428345,
0.2043602168560028,
-0.1585899144411087,
0.046571195125579834,
0.4434584677219391,
-0.22651681303977966,
0.6756607294082642,
0.27034828066825867,
-0.36859971284866333,
0.7623475790023804,
-0.03962778300046921,
0.08207204937934875,
0.06005550175905228,
0.0007318033603951335,
-0.08568822592496872,
-0.11918030679225922,
-0.1288200467824936,
0.008441757410764694,
0.7027571797370911,
0.011532580479979515,
0.19721774756908417,
-1.135250449180603,
0.4990592896938324,
-0.3692827522754669,
-0.03527327626943588,
0.4037412106990814,
0.13381020724773407,
0.34013810753822327,
-0.08368556946516037,
0.06646577268838882,
0.24103136360645294,
-0.662681519985199,
-0.19614489376544952,
0.2955757677555084,
-0.15701118111610413,
-0.09545417875051498,
0.1363838016986847,
-0.4712983965873718,
0.6125555634498596,
-0.17896729707717896,
0.82309889793396,
0.04024868458509445,
-0.22540707886219025,
-0.7031312584877014,
0.18918856978416443,
0.8676862120628357,
0.14443404972553253,
0.05626555532217026,
0.1545882672071457,
-0.04282316192984581,
0.4800279438495636,
-0.20981374382972717,
-0.1983826905488968,
0.028730100020766258,
0.24966146051883698,
0.4629918038845062,
-0.09859535098075867,
0.6437358856201172,
0.4050803482532501,
0.2815908193588257,
0.25345107913017273,
-0.22302941977977753,
0.5694441199302673,
-0.27897021174430847,
0.4791215658187866,
-0.2372768372297287,
0.0855904221534729,
0.4652259349822998,
0.38020753860473633,
0.045898471027612686,
-0.3820466101169586,
-0.7620038986206055,
-0.1091037318110466,
0.6235324144363403,
0.2249189019203186,
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] |
Material
Deposition
technique
used
Thickness
(nm)
Substrate
used
Average optical
Transmittance
(%)
Optical
band gap
(eV)
Electrical
conductivity
(S/cm)
Carrier
conc
(/cm3)
Hall
Mobility
(cm2/V-s)
FOM
(μS)
Reference
Ca3Co4O9
Spin
coating
100
Quartz
67
3
18
-
-
151
[163]
Bi2Sr2Co2Oy
PLD
50
LAO
51
3.14
181.8
5,17×1020
2.2
1350
[166]
In2O3-Ag2O
RF
Sputtering
300
Glass
20
-
113.6
4.2×1019
17
-
[167]
In2O3-MoO3
Spin
coating
80
Glass
80-88
3.8 | [
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] |
Glass
20
-
113.6
4.2×1019
17
-
[167]
In2O3-MoO3
Spin
coating
80
Glass
80-88
3.8
400
2.1×1020
11.9
-
[168]
V2O3
PLD
7-58
Sapphire
40-78
3.6
400-2122
>1022
0.14-0.24
12992
[169]
V2O3
Spray
pyrolysis
60
Sapphire
32
-
1079
2.86×1022
0.24
5699
[170]
ZnMgAlO
Spray
Pyrolysis
200
Borosilicate
glass
87.1
3.34
1
⁓1018
3.5
-
[171]
Cu-Mg (OH)2
Electro-
chemical
1000-2000
ITO coated
glass
90
4
1×10-5
-
-
-
[172]
La1-xSrxVO3
PLD
12
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chemical
1000-2000
ITO coated
glass
90
4
1×10-5
-
-
-
[172]
La1-xSrxVO3
PLD
12
LSAT
53.9–70.1
3.5
742.3–872
1.72×1021
2.1
2507-
6776
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Ballast charges for semiconductor spin qubits
Yujun Choi,1, 2, ∗ John M. Nichol,3 and Edwin Barnes1, 2
1Department of Physics, Virginia Tech, Blacksburg, VA 24061, United States
2Virginia Tech Center for Quantum Information Science and Engineering, Blacksburg, VA 24061, United States
3Department of Physics and Astronomy, University of Rochester, Rochester, NY 14627, United States
(Dated: May 24, 2024)
Semiconductor spin qubits are an attractive platform for quantum computing, but their perfor- | [
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] |
Semiconductor spin qubits are an attractive platform for quantum computing, but their perfor-
mance is degraded primarily by fluctuating electromagnetic environments. We introduce the concept
of ballast charges, which are induced charges on the surface of an additional screening layer situated
below the qubits. The counteractive behavior of these charges can significantly reduce the power
spectral density associated with fluctuations from two-level systems that contribute to charge noise. | [
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] |
Our simulations show that the dephasing time of a spin qubit in a Si/SiGe device increases by a
factor of 4 to 6 on average when using this method. We also discuss the physical implementation
and potential challenges of this approach.
Introduction — Spin qubits in semiconductor quan-
tum dots (QD) are a promising platform for quantum
computing [1]. They have reached the fidelities needed
for fault-tolerant operation [2–5] and are also compatible
with CMOS manufacturing infrastructure [6, 7]. One of | [
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] |
with CMOS manufacturing infrastructure [6, 7]. One of
the main bottlenecks for practical quantum computing
with spin qubits is pure dephasing, which typically oc-
curs on a time scale that is orders of magnitude shorter
than the spin relaxation time [8]. This dephasing is pri-
marily due to environmental noise, particularly hyperfine
noise from nearby nuclear spins of spinful isotopes and
charge noise due to random fluctuations of background
charges in QD devices [9]. Charge noise, which typically | [
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] |
charges in QD devices [9]. Charge noise, which typically
has a 1/f power spectrum [10, 11], is the dominant noise
source in silicon devices, where isotopic enrichment can
significantly reduce the density of spinful isotopes, mit-
igating hyperfine noise [12, 13]. The physical origin of
charge noise is not yet fully understood [14], but there is
evidence that two-level systems (TLSs) associated with
charge traps in an oxide layer or on the surface of a semi-
conductor layer are responsible [15–17]. | [
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] |
conductor layer are responsible [15–17].
In quantum computing, there are many approaches to
combatting environmental noise. One of them is to en-
code logical information into many physical qubits uti-
lizing quantum error correction codes, which is neces-
sary for fault-tolerant quantum computation [18, 19].
More near-term methods involve quantum error miti-
gation techniques implemented at the algorithmic level,
such as zero-noise extrapolation, probabilistic error can- | [
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] |
such as zero-noise extrapolation, probabilistic error can-
cellation, etc. [20, 21]. Other near-term error mitigation
techniques include dynamical decoupling and dynami-
cally corrected gates, decoherence-free subspaces, active
feedforward loops, and tuning to sweet spots in the pa-
rameter space of a particular qubit device [22–25].
In this Letter, we introduce an alternative approach
to reducing the effect of charge noise in QD spin qubits
that makes use of ballast charges in the device. The con- | [
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that makes use of ballast charges in the device. The con-
cept of ballast charges originates from the idea of ballast
water used for maritime vessels.
In that context, bal-
last water is used to control the buoyant force acting
on vessels to improve their stability and maneuverability
in various maritime conditions; for example, the loading
of heavy ballast water can provide added stability when
bad weather is expected [26]. Analogously, our central
idea is to use ballast charges to make spin qubits less | [
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] |
idea is to use ballast charges to make spin qubits less
susceptible to charge noise, leading to an increase in the
dephasing time of the qubits. The underlying principle of
ballast charges relies on electrostatic induction, where in-
duced charges are redistributed to counteract the change
in electric fields that are external to the charges. Hence,
the ballast charges for spin qubits should be a kind of
induced charge that can move freely to compensate for
the fluctuations of TLSs. | [
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induced charge that can move freely to compensate for
the fluctuations of TLSs.
This approach can also be regarded as leveraging the
screening effect of additional electrons in the device. A
recent experimental study indirectly exhibits the screen-
ing effect by adding electrons to a charge sensor close
to a QD [27].
Other studies show that the coherence
of a spin qubit can be enhanced when the qubit is de-
fined with multiple electrons in a QD [28, 29]. In such | [
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] |
fined with multiple electrons in a QD [28, 29]. In such
a scheme, however, we can only expect a small screening
effect from induction because the electrons are strongly
confined within the QD. Furthermore, the extra electrons
complicate gate operations due to the inherent complex-
ity (large Hilbert space) of the multi-electron qubit. This
suggests that ballast charges should be extrinsic to the
QD and to the qubit itself.
One possible way to introduce more mobile ballast | [
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] |
QD and to the qubit itself.
One possible way to introduce more mobile ballast
charges is to insert a metallic layer below the quantum
well (QW) in which the 2D electron gas (2DEG) that is
used to form the qubits resides. This is a natural choice
in terms of electrostatic induction. Alternatively, an ad-
ditional 2DEG can also be used for this purpose, as this
would also allow electrons to move freely. For now, we
suppose that there is an additional layer in the device | [
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] |
suppose that there is an additional layer in the device
that can host ballast charges, and the merits and draw-
backs of different physical implementations will be dis-
cussed later.
A schematic diagram for ballast charges in a Si/SiGe
QD device is shown in Fig. 1(a). A screening layer is
arXiv:2405.14027v1 [cond-mat.mes-hall] 22 May 2024
2
QD
TLS
Ballast charges
SiGe
SiGe
Oxide
Gate
𝑥𝑥
𝑧𝑧
TLS
SiGe
Oxide
Gate
𝑥𝑥
𝑧𝑧
Image TLS
(a)
(b)
SiGe
SiGe
SiGe
𝐵𝐵𝑄𝑄
𝐸𝐸𝑥𝑥
𝐸𝐸𝑧𝑧
QD
Si QW
𝑧𝑧 = 0
𝑑𝑑
Si QW | [
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] |
TLS
SiGe
Oxide
Gate
𝑥𝑥
𝑧𝑧
Image TLS
(a)
(b)
SiGe
SiGe
SiGe
𝐵𝐵𝑄𝑄
𝐸𝐸𝑥𝑥
𝐸𝐸𝑧𝑧
QD
Si QW
𝑧𝑧 = 0
𝑑𝑑
Si QW
FIG. 1. Schematic diagrams for ballast charges in a Si/SiGe quantum dot device. (a) Ballast charges are induced charges due
to TLSs (red ±) and gate voltages (orange ±). The ballast charges are on the surface of the additional screening layer below
thin Si quantum well and SiGe layers. (b) Different viewpoint for ballast charges using the method of image charges. The | [
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] |
electric fields (Ex and Ez) at the QD position come from TLSs (solid arrows) and their image TLSs (dashed arrows). The
diagrams are not to scale. Si cap between the SiGe and oxide layers and micromagnets on top of the gate layer are not shown.
inserted below a thin SiGe layer that confines a QD in
the Si QW. The QD plane is defined as z = 0, and the
distance between the QD plane and the screening layer is
d. There are two kinds of ballast charges on the surface of | [
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] |
d. There are two kinds of ballast charges on the surface of
the screening layer: One is due to TLSs (red ±) and the
other is due to applied gate voltages (orange ±) where ±
denote positive and negative charges on the surface of the
screening layer respectively. The ballast charges due to
TLSs are the key to the suppression of charge noise since
they compensate for the change in electric potential or
field at the QD via redistribution. If a TLS is modeled as | [
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] |
field at the QD via redistribution. If a TLS is modeled as
a flipping electric dipole whose position and orientation
are fixed, the ballast charges will change their signs as
the TLS flips back and forth. The ballast charges due to
gate voltages can be taken into account as offsets when
calibrating and tuning the device in the first place.
The role of ballast charges can be understood by the
method of image charges as shown in Fig. 1(b). An im-
age TLS corresponding to the TLS in the oxide layer is | [
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] |
age TLS corresponding to the TLS in the oxide layer is
illustrated as dashed red arrows. Assuming the screening
layer is much larger than the size of the QD and TLS and
exactly located at the QD plane, the horizontal compo-
nents of the electric field due to the real and image TLSs
perfectly cancel out, while the vertical component is dou-
bled. This gives rise to zero detuning noise provided that
there is an in-plane external magnetic field (BQ), and the | [
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] |
there is an in-plane external magnetic field (BQ), and the
dominant magnetic field gradients due to micromagnets
are ∂BQ/∂x and ∂BQ/∂y.
However, this is not what
we want, because the qubit cannot be defined due to the
equipotential surface along the QD plane. Moreover, it is
not possible to make the screening layer at the QD plane
in practice. Only partial cancellation of the charge noise
will appear when the screening layer is a finite distance
away from the QD plane (see Supplemental Material for | [
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] |
away from the QD plane (see Supplemental Material for
an analytical result on this).
Results — Examples of simulated power spectral den-
sities (PSDs) are shown for the electric potential and the
spin qubit precession frequency in Figs.
2(a) and (b),
respectively.
TLSs are assumed to be at the interface
of the oxide and gate layers (z = 50 nm) with random
orientations.
The orders of magnitude of the PSD for
the spin qubit frequency agree well with the experimen- | [
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] |
The orders of magnitude of the PSD for
the spin qubit frequency agree well with the experimen-
tal data in Ref. [13]. As expected, the reduction in the
PSDs increases as the screening layer is located closer to
the QD plane from z = −15 to z = −5 nm. For a 10
nm Si QW, which is a typical width for realistic devices,
the PSD for the electric potential is decreased by about
two orders of magnitude. If we make thin Si QW and
SiGe layers of 5 nm thickness each [27], the PSD can be | [
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] |
SiGe layers of 5 nm thickness each [27], the PSD can be
reduced by about three orders of magnitude. The reduc-
tion in the PSD for the spin qubit frequency is less than
that for the electric potential, which is about two orders
of magnitude for d = 5 nm. This can be attributed to
the vector property of compensating electric fields that
are more sensitive to the positions and orientations of the
image TLSs in the device.
The dephasing time of the qubit can be directly com- | [
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0.21876683831214905
] |
image TLSs in the device.
The dephasing time of the qubit can be directly com-
puted from the PSD for the spin qubit frequency as-
3
(a)
(b)
No sc.
Sc. at z=-15 nm
Sc. at z=-10 nm
Sc. at z=-5 nm
10-5
10-4
10-3
10-2
10-1
10-14
10-11
10-8
10-5
PSD (V2/Hz)
No sc.
Sc. at z=-15 nm
Sc. at z=-10 nm
Sc. at z=-5 nm
10-5
10-4
10-3
10-2
10-1
107
1010
1013
1016
Frequency (Hz)
PSD (Hz2/Hz)
FIG. 2. An example of simulated power spectral densities for
(a) electric potential and (b) spin qubit frequency for several | [
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] |
(a) electric potential and (b) spin qubit frequency for several
distances d between the QD and screening layer (Sc. at z =
−d). The case of no screening layer (No sc.) is also shown.
suming Gaussian noise [30]. The dephasing times for no
screening, screening at z = −15 nm, z = −10 nm, and
z = −5 nm are 2.1, 7.5, 11.7, and 25.2 µs, respectively.
This enhancement can be understood from the relation
T ∗
2 ∼ 1/
��
S(ω)dω in the quasistatic limit [27].
The
simulation parameters and details are given in the Sup- | [
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